[Science Journal Cover design] Enhanced and Eco-Friendly Recycling of Carbon-Fiber-Reinforced Plastics Using Water at Ambient Pressure

Science Journal Cover

Cross-linked epoxy resin, a thermosetting resin, typically cannot be dissolved in organic solvents, making materials like carbon-fiber-reinforced plastics (CFRPs) challenging to recycle. Our study has successfully dissolved epoxy resin within 2 hours at atmospheric pressure and 100 °C, the optimal conditions for depolymerization, using an aqueous NaOCl solution. This breakthrough enables the recycling of CFRPs. The depolymerization mechanism involves hydroxyl radicals generated from the aqueous NaOCl solution. We identified that an initial pH of 12.05 and a reaction temperature of 100 °C are ideal for the process. The reclaimed carbon fibers (CFs) maintained physical properties similar to those of virgin CFs. Additionally, high-value products were fabricated using the CFs and resin decomposition products recovered after CFRP decomposition, maximizing recyclability and minimizing waste generation. -Journal cover design by scapiens

https://pubs.acs.org/doi/10.1021/acssuschemeng.9b06371

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